Like has been said already, the holes are offset, so enlarging the existing hole won't work.
Daniel Defense sells large hole flat top uppers, that would be your easiest solution. Another alternative that I've seen pictures of is to fill the holes on the lower with aluminum rod, pinned to ensure they don't move, and then drill the small hole in the proper location. You'd still need the two part screw (they make a small version) because the lower won't be able to retain the pivot pin.